The road that connects Vasilissis Amalias with Filopappou is the perfect opportunity for pedestrians to walk, chill and chat, offering a view of Acropolis. Locals most of the times prefer to walk the part that connects Thiseio with Acropolis, a choice that I also recommend!
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Apart from the fact that Dionysiou Aeropagitou is connecting the ancient market with Acropolis, passing through the neighborhood of Makrigianni, full of manor houses, walking through this street is about to fill you with Athens most positive vibes. Street artists and some ice cream during spring, make the experience even better.
Somewhere near Filopappou you'll find some steps leading to Irodio, do not forget to visit!